This will result in positive charge accumulation on -R-NH 3 +, and thus stronger Coulomb force of bond (-R-NH 3 +)-(PbBr 4 2−), which facilitates excitons self-trapping. The halogen-substituents will withdraw electrons from the branched chain (-R-NH 3 +) of the phenyl molecule. Halogen-substituted phenyl molecules are applied to synthesize perovskite crystals. Here, we report an atom-substituting strategy to trigger STEs formation in layered perovskites. Since the mechanism of STEs formation in perovskites is still not clear, preparing new low-dimensional white perovskites relies mostly on screening lots of intercalated organic molecules rather than rational design. The broadband white emission originates from self-trapped excitons (STEs). Low-dimensional hybrid perovskites have demonstrated excellent performance as white-light emitters.
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